Impurity-Induced Plasmon Damping in Individual Cobalt-Doped Hollow Au Nanoshells

dc.citation.journalTitleThe Journal of Physical Chemistry Ben_US
dc.contributor.authorThibodeaux, Christyn A.en_US
dc.contributor.authorKulkarni, Vikramen_US
dc.contributor.authorChang, Wei-Shunen_US
dc.contributor.authorNeumann, Oaraen_US
dc.contributor.authorCao, Yangen_US
dc.contributor.authorBrinson, Bruceen_US
dc.contributor.authorAyala-Orozco, Ciceronen_US
dc.contributor.authorChen, Chih-Weien_US
dc.contributor.authorMorosan, Emiliaen_US
dc.contributor.authorLink, Stephanen_US
dc.contributor.authorNordlander, Peteren_US
dc.contributor.authorHalas, Naomi J.en_US
dc.contributor.orgLaboratory for Nanophotonicsen_US
dc.contributor.orgRice Quantum Instituteen_US
dc.date.accessioned2014-07-23T15:30:36Z
dc.date.available2014-07-23T15:30:36Z
dc.date.issued2014en_US
dc.description.abstractThe optical properties of plasmonic nanoparticles in the size range corresponding to the electrostatic, or dipole, limit have the potential to reveal effects otherwise masked by phase retardation. Here we examine the optical properties of individual, sub-50 nm hollow Au nanoshells (Co-HGNS), where Co is the initial sacrificial core nanoparticle, using single particle total internal reflection scattering (TIRS) spectroscopy. The residual Co present in the metallic shell induces a substantial broadening of the homogeneous plasmon resonance line width of the Co-HGNS, where the full width at half-maximum (fwhm) broadens proportionately with increasing Co content. This doping-induced line broadening provides a strategy for controlling plasmon line width independent of nanoparticle size, and has the potential to substantially modify the relative decay channels for localized nanoparticle surface plasmons.en_US
dc.identifier.citationThibodeaux, Christyn A., Kulkarni, Vikram, Chang, Wei-Shun, et al.. "Impurity-Induced Plasmon Damping in Individual Cobalt-Doped Hollow Au Nanoshells." <i>The Journal of Physical Chemistry B,</i> (2014) American Chemical Society: http://dx.doi.org/10.1021/jp504467j.
dc.identifier.doihttp://dx.doi.org/10.1021/jp504467jen_US
dc.identifier.urihttps://hdl.handle.net/1911/76262
dc.language.isoengen_US
dc.publisherAmerican Chemical Society
dc.rightsThis is an author's peer-reviewed final manuscript, as accepted by the publisher. The published article is copyrighted by the American Chemical Society.en_US
dc.titleImpurity-Induced Plasmon Damping in Individual Cobalt-Doped Hollow Au Nanoshellsen_US
dc.typeJournal articleen_US
dc.type.dcmiTexten_US
dc.type.publicationpost-printen_US
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