Midinfrared third-harmonic generation from macroscopically aligned ultralong single-wall carbon nanotubes
| dc.citation.firstpage | 161405(R) | en_US |
| dc.citation.journalTitle | Physical Review B | en_US |
| dc.citation.volumeNumber | 87 | en_US |
| dc.contributor.author | Morris, D.T. | en_US |
| dc.contributor.author | Pint, C.L. | en_US |
| dc.contributor.author | Arvidson, R.S. | en_US |
| dc.contributor.author | Luttge, A. | en_US |
| dc.contributor.author | Hauge, R.H. | en_US |
| dc.contributor.author | Belyanin, A.A. | en_US |
| dc.contributor.author | Woods, G.L. | en_US |
| dc.contributor.author | Kono, J. | en_US |
| dc.date.accessioned | 2013-05-02T17:04:00Z | en_US |
| dc.date.available | 2013-05-02T17:04:00Z | en_US |
| dc.date.issued | 2013 | en_US |
| dc.description.abstract | We report the observation of strong third-harmonic generation from a macroscopic array of aligned ultralong single-wall carbon nanotubes (SWCNTs)with intensemidinfrared radiation. Through power-dependent experiments, we determined the absolute value of the third-order nonlinear optical susceptibility !(3) of our SWCNT film to be 5.53 × 10−12 esu, three orders of magnitude larger than that of the fused silica reference we used. Taking account of the filling factor of 8.75% for our SWCNT film, we estimate a !(3) of 6.32 × 10−11 esu for a fully dense film. Furthermore, through polarization-dependent experiments, we extracted all the nonzero elements of the !(3) tensor, determining the magnitude of the weaker tensor elements to be #1/6 of that of the dominant !(3) zzzz component. | en_US |
| dc.embargo.terms | none | en_US |
| dc.identifier.citation | Morris, D.T., Pint, C.L., Arvidson, R.S., et al.. "Midinfrared third-harmonic generation from macroscopically aligned ultralong single-wall carbon nanotubes." <i>Physical Review B,</i> 87, (2013) American Physical Society: 161405(R). http://dx.doi.org/10.1103/PhysRevB.87.161405. | en_US |
| dc.identifier.doi | http://dx.doi.org/10.1103/PhysRevB.87.161405 | en_US |
| dc.identifier.uri | https://hdl.handle.net/1911/71090 | en_US |
| dc.language.iso | eng | en_US |
| dc.publisher | American Physical Society | en_US |
| dc.rights | Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. | en_US |
| dc.title | Midinfrared third-harmonic generation from macroscopically aligned ultralong single-wall carbon nanotubes | en_US |
| dc.type | Journal article | en_US |
| dc.type.dcmi | Text | en_US |
| dc.type.publication | publisher version | en_US |