Wiess School of Natural Sciences

Permanent URI for this community

https://hdl.handle.net/1911/17012

Browse

Browsing Wiess School of Natural Sciences by Author "Abernathy, D.L."

Now showing 1 - 5 of 5
  • Thumbnail Image
    Item
    Coexistence of Ferromagnetic and Stripe Antiferromagnetic Spin Fluctuations in SrCo2As2
    (American Physical Society, 2019) Li, Yu; Yin, Zhiping; Liu, Zhonghao; Wang, Weiyi; Xu, Zhuang; Song, Yu; Tian, Long; Huang, Yaobo; Shen, Dawei; Abernathy, D.L.; Niedziela, J.L.; Ewings, R.A.; Perring, T.G.; Pajerowski, Daniel M.; Matsuda, Masaaki; Bourges, Philippe; Mechthild, Enderle; Su, Yixi; Dai, Pengcheng
    We use inelastic neutron scattering to study energy and wave vector dependence of spin fluctuations in SrCo2As2, derived from SrFe2−xCoxAs2 iron pnictide superconductors. Our data reveal the coexistence of antiferromagnetic (AF) and ferromagnetic (FM) spin fluctuations at wave vectors QAF=(1,0) and QFM=(0,0)/(2,0), respectively. By comparing neutron scattering results with those of dynamic mean field theory calculation and angle-resolved photoemission spectroscopy experiments, we conclude that both AF and FM spin fluctuations in SrCo2As2 are closely associated with a flatband of the eg orbitals near the Fermi level, different from the t2g orbitals in superconducting SrFe2−xCoxAs2. Therefore, Co substitution in SrFe2−xCoxAs2 induces a t2g to eg orbital switching, and is responsible for FM spin fluctuations detrimental to the singlet pairing superconductivity.
  • Thumbnail Image
    Item
    Effect of Pnictogen Height on Spin Waves in Iron Pnictides
    (American Physical Society, 2014) Zhang, Chenglin; Harriger, Leland W.; Yin, Zhiping; Lv, Weicheng; Wang, Miaoyin; Tan, Guotai; Song, Yu; Abernathy, D.L.; Tian, Wei; Egami, Takeshi; Haule, Kristjan; Kotliar, Gabriel; Dai, Pengcheng
    We use inelastic neutron scattering to study spin waves in the antiferromagnetic ordered phase of iron pnictide NaFeAs throughout the Brillouin zone. Comparing with the well-studied AFe2As2 (A=Ca, Sr, Ba) family, spin waves in NaFeAs have considerably lower zone boundary energies and more isotropic effective in-plane magnetic exchange couplings. These results are consistent with calculations from a combined density functional theory and dynamical mean field theory and provide strong evidence that pnictogen height controls the strength of electron-electron correlations and consequently the effective bandwidth of magnetic excitations.
  • Thumbnail Image
    Item
    Electron doping evolution of the magnetic excitations in NaFe1−xCoxAs
    (American Physical Society, 2016) Carr, Scott V.; Zhang, Chenglin; Song, Yu; Tan, Guotai; Li, Yu; Abernathy, D.L.; Stone, M.B.; Granroth, G.E.; Perring, T.G.; Dai, Pengcheng
    We use time-of-flight (TOF) inelastic-neutron-scattering (INS) spectroscopy to investigate the doping dependence of magnetic excitations across the phase diagram of NaFe 1 − x Co x As with x = 0 , 0.0175, 0.0215, 0.05, and 0.11 . The effect of electron doping by partially substituting Fe by Co is to form resonances that couple with superconductivity, broaden, and suppress low-energy ( E ≤ 80 meV) spin excitations compared with spin waves in undoped NaFeAs. However, high-energy ( E > 80 meV) spin excitations are weakly Co-doping-dependent. Integration of the local spin dynamic susceptibility χ ' ' ( ω ) of NaFe 1 − x Co x As reveals a total fluctuating moment of 3.6 μ 2 B /Fe and a small but systematic reduction with electron doping. The presence of a large spin gap in Co-overdoped nonsuperconducting NaFe 0.89 Co 0.11 As suggests that Fermi surface nesting is responsible for low-energy spin excitations. These results parallel the Ni-doping evolution of spin excitations in BaFe 2 − x Ni x As 2 in spite of the differences in crystal structures and Fermi surface evolution in these two families of iron pnictides, thus confirming the notion that low-energy spin excitations coupling with itinerant electrons are important for superconductivity, while weakly doping-dependent high-energy spin excitations result from localized moments.
  • Thumbnail Image
    Item
    Energy dependence of the spin excitation anisotropy in uniaxial-strained BaFe1.9Ni0.1As2
    (American Physical Society, 2015) Song, Yu; Lu, Xingye; Abernathy, D.L.; Tam, David W.; Niedziela, J.L.; Tian, Wei; Luo, Huiqian; Si, Qimiao; Dai, Pengcheng
    We use inelastic neutron scattering to study the temperature and energy dependence of the spin excitation anisotropy in uniaxial-strained electron-doped iron pnictide BaFe1.9Ni0.1As2 near optimal superconductivity (Tc=20K). Our work has been motivated by the observation of in-plane resistivity anisotropy in the paramagnetic tetragonal phase of electron-underdoped iron pnictides under uniaxial pressure, which has been attributed to a spin-driven Ising-nematic state or orbital ordering. Here we show that the spin excitation anisotropy, a signature of the spin-driven Ising-nematic phase, exists for energies below ∼60 meV in uniaxial-strained BaFe1.9Ni0.1As2. Since this energy scale is considerably larger than the energy splitting of the dxz and dyz bands of uniaxial-strained Ba(Fe1−xCox)2As2 near optimal superconductivity, spin Ising-nematic correlations are likely the driving force for the resistivity anisotropy and associated electronic nematic correlations.
  • Thumbnail Image
    Item
    Orbital Selective Spin Excitations and their Impact on Superconductivity of LiFe1−xCoxAs
    (American Physical Society, 2016) Li, Yu; Yin, Zhiping; Wang, Xiancheng; Tam, David W.; Abernathy, D.L.; Podlesnyak, A.; Zhang, Chenglin; Wang, Meng; Xing, Lingyi; Jin, Changqing; Haule, Kristjan; Kotliar, Gabriel; Maier, Thomas A.; Dai, Pengcheng
    We use neutron scattering to study spin excitations in single crystals of LiFe0.88Co0.12As, which is located near the boundary of the superconducting phase of LiFe1−xCoxAs and exhibits non-Fermi-liquid behavior indicative of a quantum critical point. By comparing spin excitations of LiFe0.88Co0.12As with a combined density functional theory and dynamical mean field theory calculation, we conclude that wave-vector correlated low energy spin excitations are mostly from the dxy orbitals, while high-energy spin excitations arise from the dyz and dxz orbitals. Unlike most iron pnictides, the strong orbital selective spin excitations in the LiFeAs family cannot be described by an anisotropic Heisenberg Hamiltonian. While the evolution of low-energy spin excitations of LiFe1−xCoxAs is consistent with the electron-hole Fermi surface nesting conditions for the dxy orbital, the reduced superconductivity in LiFe0.88Co0.12As suggests that Fermi surface nesting conditions for the dyz and dxz orbitals are also important for superconductivity in iron pnictides.