Enhancing the photocurrent and photoluminescence of single crystal monolayer MoS2ᅠwith resonant plasmonic nanoshells

Abstract

Monolayer molybdenum disulfide (MoS2) produced by controlled vapor-phase synthesis is a commercially promising new two-dimensional material for optoelectronics because of its direct bandgap and broad absorption in the visible and ultraviolet regimes. By tuning plasmonic core-shell nanoparticles to the direct bandgap of monolayer MoS2 and depositing them sparsely (<1% coverage) onto the material's surface, we observe a threefold increase in photocurrent and a doubling of photoluminescence signal for both excitonic transitions, amplifying but not altering the intrinsic spectral response.

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Sobhani, Ali, Lauchner, Adam, Najmaei, Sina, et al.. "Enhancing the photocurrent and photoluminescence of single crystal monolayer MoS2ᅠwith resonant plasmonic nanoshells." Applied Physics Letters, 104, no. 3 (2014) AIP Publishing LLC.: http://dx.doi.org/10.1063/1.4862745.

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