Generation of intense phase-stable femtosecond hard X-ray pulse pairs

dc.citation.articleNumbere2119616119
dc.citation.issueNumber12
dc.citation.journalTitleProceedings of the National Academy of Sciences
dc.citation.volumeNumber119
dc.contributor.authorZhang, Yu
dc.contributor.authorKroll, Thomas
dc.contributor.authorWeninger, Clemens
dc.contributor.authorMichine, Yurina
dc.contributor.authorFuller, Franklin D.
dc.contributor.authorZhu, Diling
dc.contributor.authorAlonso-Mori, Roberto
dc.contributor.authorSokaras, Dimosthenis
dc.contributor.authorLutman, Alberto A.
dc.contributor.authorHalavanau, Aliaksei
dc.contributor.authorPellegrini, Claudio
dc.contributor.authorBenediktovitch, Andrei
dc.contributor.authorYabashi, Makina
dc.contributor.authorInoue, Ichiro
dc.contributor.authorInubushi, Yuichi
dc.contributor.authorOsaka, Taito
dc.contributor.authorYamada, Jumpei
dc.contributor.authorBabu, Ganguli
dc.contributor.authorSalpekar, Devashish
dc.contributor.authorSayed, Farheen N.
dc.contributor.authorAjayan, Pulickel M.
dc.contributor.authorKern, Jan
dc.contributor.authorYano, Junko
dc.contributor.authorYachandra, Vittal K.
dc.contributor.authorYoneda, Hitoki
dc.contributor.authorRohringer, Nina
dc.contributor.authorBergmann, Uwe
dc.date.accessioned2022-04-15T14:45:34Z
dc.date.available2022-04-15T14:45:34Z
dc.date.issued2022
dc.description.abstractCoherent nonlinear spectroscopies and imaging in the X-ray domain provide direct insight into the coupled motions of electrons and nuclei with resolution on the electronic length scale and timescale. The experimental realization of such techniques will strongly benefit from access to intense, coherent pairs of femtosecond X-ray pulses. We have observed phase-stable X-ray pulse pairs containing more than 3 × 107 photons at 5.9 keV (2.1 Å) with ∼1 fs duration and 2 to 5 fs separation. The highly directional pulse pairs are manifested by interference fringes in the superfluorescent and seeded stimulated manganese Kα emission induced by an X-ray free-electron laser. The fringes constitute the time-frequency X-ray analog of Young’s double-slit interference, allowing for frequency domain X-ray measurements with attosecond time resolution.
dc.identifier.citationZhang, Yu, Kroll, Thomas, Weninger, Clemens, et al.. "Generation of intense phase-stable femtosecond hard X-ray pulse pairs." <i>Proceedings of the National Academy of Sciences,</i> 119, no. 12 (2022) National Academy of Sciences: https://doi.org/10.1073/pnas.2119616119.
dc.identifier.digitalpnas-2119616119
dc.identifier.doihttps://doi.org/10.1073/pnas.2119616119
dc.identifier.urihttps://hdl.handle.net/1911/112096
dc.language.isoeng
dc.publisherNational Academy of Sciences
dc.rightsThis article is distributed under Creative Commons Attribution-NonCommercial-NoDerivatives License 4.0 (CC BY-NC-ND)
dc.rights.urihttps://creativecommons.org/licenses/by-nc-nd/4.0/
dc.titleGeneration of intense phase-stable femtosecond hard X-ray pulse pairs
dc.typeJournal article
dc.type.dcmiText
dc.type.publicationpublisher version
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