In structural vibration response sensing, mobile sensors offer outstanding benefits as they are not dedicated to a certain structure; they also possess the ability to acquire dense spatial information. Currently, most of the existing literature concerning mobile sensing involves human drivers manually driving through the bridges multiple times. While self-driving automated vehicles could serve for such studies, they might entail substantial costs when applied to structural health monitoring tasks. Therefore, in order to tackle this challenge, we introduce a formation control framework that facilitates automatic multi-agent mobile sensing. Notably, our findings demonstrate that the proposed formation control algorithm can effectively control the behavior of the multi-agent systems for structural response sensing purposes based on user choice. We leverage vibration data collected by these mobile sensors to estimate the full-field vibration response of the structure, utilizing a compressive sensing algorithm in the spatial domain. The task of estimating the full-field response can be represented as a spatiotemporal response matrix completion task, wherein the suite of multi-agent mobile sensors sparsely populates some of the matrix’s elements. Subsequently, we deploy the compressive sensing technique to obtain the dense full-field vibration complete response of the structure and estimate the reconstruction accuracy. Results obtained from two different formations on a simply supported bridge are presented in this paper, and the high level of accuracy in reconstruction underscores the efficacy of our proposed framework. This multi-agent mobile sensing approach showcases the significant potential for automated structural response measurement, directly applicable to health monitoring and resilience assessment objectives.