Insights on synergy of materials and structures in biomimetic platelet-matrix composites

dc.citation.articleNumber051601en_US
dc.citation.issueNumber5en_US
dc.citation.journalTitleApplied Physics Lettersen_US
dc.citation.volumeNumber112en_US
dc.contributor.authorSakhavand, Naviden_US
dc.contributor.authorShahsavari, Rouzbehen_US
dc.contributor.orgSmalley Institute for Nanoscale Science and Technologyen_US
dc.date.accessioned2018-07-11T17:18:36Zen_US
dc.date.available2018-07-11T17:18:36Zen_US
dc.date.issued2018en_US
dc.description.abstractHybrid materials such as biomimetic platelet-matrix composites are in high demand to confer low weight and multifunctional mechanical properties. This letter reports interfacial-bond regulated assembly of polymers on cement-an archetype model with significant infrastructure applications. We demonstrate a series of 20+ molecular dynamics studies on decoding and optimizing the complex interfacial interactions including the role and types of various heterogeneous, competing interfacial bonds that are key to adhesion and interfacial strength. Our results show an existence of an optimum overlap length scale (∼15 nm) between polymers and cement crystals, exhibiting the best balance of strength, toughness, stiffness, and ductility for the composite. This finding, combined with the fundamental insights into the nature of interfacial bonds, provides key hypotheses for selection and processing of constituents to deliberate the best synergy in the structure and materials of platelet-matrix composites.en_US
dc.identifier.citationSakhavand, Navid and Shahsavari, Rouzbeh. "Insights on synergy of materials and structures in biomimetic platelet-matrix composites." <i>Applied Physics Letters,</i> 112, no. 5 (2018) AIP Publishing: https://doi.org/10.1063/1.5017200.en_US
dc.identifier.doihttps://doi.org/10.1063/1.5017200en_US
dc.identifier.urihttps://hdl.handle.net/1911/102382en_US
dc.language.isoengen_US
dc.publisherAIP Publishingen_US
dc.rightsArticle is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use.en_US
dc.titleInsights on synergy of materials and structures in biomimetic platelet-matrix compositesen_US
dc.typeJournal articleen_US
dc.type.dcmiTexten_US
dc.type.publicationpublisher versionen_US
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