Browsing by Author "Stone, M.B."

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    Electron doping evolution of the magnetic excitations in NaFe1−xCoxAs
    (American Physical Society, 2016) Carr, Scott V.; Zhang, Chenglin; Song, Yu; Tan, Guotai; Li, Yu; Abernathy, D.L.; Stone, M.B.; Granroth, G.E.; Perring, T.G.; Dai, Pengcheng
    We use time-of-flight (TOF) inelastic-neutron-scattering (INS) spectroscopy to investigate the doping dependence of magnetic excitations across the phase diagram of NaFe 1 − x Co x As with x = 0 , 0.0175, 0.0215, 0.05, and 0.11 . The effect of electron doping by partially substituting Fe by Co is to form resonances that couple with superconductivity, broaden, and suppress low-energy ( E ≤ 80 meV) spin excitations compared with spin waves in undoped NaFeAs. However, high-energy ( E > 80 meV) spin excitations are weakly Co-doping-dependent. Integration of the local spin dynamic susceptibility χ ' ' ( ω ) of NaFe 1 − x Co x As reveals a total fluctuating moment of 3.6 μ 2 B /Fe and a small but systematic reduction with electron doping. The presence of a large spin gap in Co-overdoped nonsuperconducting NaFe 0.89 Co 0.11 As suggests that Fermi surface nesting is responsible for low-energy spin excitations. These results parallel the Ni-doping evolution of spin excitations in BaFe 2 − x Ni x As 2 in spite of the differences in crystal structures and Fermi surface evolution in these two families of iron pnictides, thus confirming the notion that low-energy spin excitations coupling with itinerant electrons are important for superconductivity, while weakly doping-dependent high-energy spin excitations result from localized moments.
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    Evolution of Magnetic Double Helix and Quantum Criticality near a Dome of Superconductivity in CrAs
    (American Physical Society, 2018) Matsuda, M.; Lin, F.K.; Yu, R.; Cheng, J.-G.; Wu, W.; Sun, J.P.; Zhang, J.H.; Sun, P.J.; Matsubayashi, K.; Miyake, T.; Kato, T.; Yan, J.-Q.; Stone, M.B.; Si, Qimiao; Luo, J.L.; Uwatoko, Y.
    At ambient pressure, CrAs undergoes a first-order transition into a double-helical magnetic state at TN=265  K, which is accompanied by a structural transition. The recent discovery of pressure-induced superconductivity in CrAs makes it important to clarify the nature of quantum phase transitions out of the coupled structural/helimagnetic order in this system. Here, we show, via neutron diffraction on the single-crystal CrAs under hydrostatic pressure (P), that the combined order is suppressed at Pc≈10  kbar, near which bulk superconductivity develops with a maximal transition temperature Tc≈2  K. We further show that the coupled order is also completely suppressed by phosphorus doping in CrAs1−xPx at a critical xc≈0.05, above which inelastic neutron scattering evidenced persistent antiferromagnetic correlations, providing a possible link between magnetism and superconductivity. In line with the presence of antiferromagnetic fluctuations near Pc(xc), the A coefficient of the quadratic temperature dependence of resistivity exhibits a dramatic enhancement as P (x) approaches Pc(xc), around which ρ(T) has a non-Fermi-liquid form. Accordingly, the electronic specific-heat coefficient of CrAs1−xPx peaks around xc. These properties provide clear evidence for quantum criticality, which we interpret as originating from a nearly second-order helimagnetic quantum phase transition that is concomitant with a first-order structural transition. Our findings in CrAs highlight the distinct characteristics of quantum criticality in bad metals, thereby bringing out new insights into the physics of unconventional superconductivity such as those occurring in the high-Tc iron pnictides.