Browsing by Author "Niedermayer, Christof"

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    Doping effects of Cr on the physical properties of BaFe1.9−xNi0.1CrxAs2
    (American Physical Society, 2018) Gong, Dongliang; Xie, Tao; Zhang, Rui; Birk, Jonas; Niedermayer, Christof; Han, Fei; Lapidus, S.H.; Dai, Pengcheng; Li, Shiliang; Luo, Huiqian
    We present a systematic study on the heavily Cr doped iron pnictides BaFe1.9−xNi0.1CrxAs2 by using elastic neutron scattering, high-resolution synchrotron x-ray diffraction (XRD), resistivity, and Hall transport measurements. When the Cr concentration increases from x=0 to 0.8, neutron diffraction experiments suggest that the collinear antiferromagnetism persists in the whole doping range, where the Néel temperature TN coincides with the tetragonal-to-orthorhombic structural transition temperature Ts, and both of them keeps around 35 K. The magnetic ordered moment, on the other hand, increases within increasing x until x=0.5, and then decreases with further increasing x. Detailed refinement of the powder XRD patterns reveals that the Cr substitutions actually stretch the FeAs4 tetrahedron along the c axis and lift the arsenic height away from the Fe-Fe plane. Transport results indicate that the charge carriers become more localized upon Cr doping, then changes from electron type to hole type around x=0.5. Our results suggest that the ordered moment and the ordered temperature of static magnetism in iron pnictides can be decoupled and tuned separately by chemical doping.
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    Doping evolution of antiferromagnetism and transport properties in nonsuperconducting BaFe2−2xNixCrxAs2
    (American Physical Society, 2015) Zhang, Rui; Gong, Dongliang; Lu, Xingye; Li, Shiliang; Laver, Mark; Niedermayer, Christof; Danilkin, Sergey; Deng, Guochu; Dai, Pengcheng; Luo, Huiqian
    We report elastic neutron scattering and transport measurements on the Ni and Cr equivalently doped iron pnictide BaFe2−2xNixCrxAs2. Compared with the electron-doped BaFe2−xNixAs2, the long-range antiferromagnetic (AF) order in BaFe2−2xNixCrxAs2 is gradually suppressed with vanishing ordered moment and Néel temperature near x=0.20 without the appearance of superconductivity. A detailed analysis on the transport properties of BaFe2−xNixAs and BaFe2−2xNixCrxAs2 suggests that the non-Fermi-liquid behavior associated with the linear resistivity as a function of temperature may not correspond to the disappearance of the static AF order. From the temperature dependence of the resistivity in overdoped compounds without static AF order, we find that the transport properties are actually affected by Cr impurity scattering, which may induce a metal-to-insulator crossover in highly doped BaFe1.7−yNi0.3CryAs2.
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    Doping evolution of antiferromagnetism and transport properties in nonsuperconducting BaFe2−2xNixCrxAs2
    (American Physical Society, 2015) Zhang, Rui; Gong, Dongliang; Lu, Xingye; Li, Shiliang; Laver, Mark; Niedermayer, Christof; Danilkin, Sergey; Deng, Guochu; Dai, Pengcheng; Luo, Huiqian
    We report elastic neutron scattering and transport measurements on the Ni and Cr equivalently doped iron pnictide BaFe2−2xNixCrxAs2. Compared with the electron-doped BaFe2−xNixAs2, the long-range antiferromagnetic (AF) order in BaFe2−2xNixCrxAs2 is gradually suppressed with vanishing ordered moment and Néel temperature near x=0.20 without the appearance of superconductivity. A detailed analysis on the transport properties of BaFe2−xNixAs and BaFe2−2xNixCrxAs2 suggests that the non-Fermi-liquid behavior associated with the linear resistivity as a function of temperature may not correspond to the disappearance of the static AF order. From the temperature dependence of the resistivity in overdoped compounds without static AF order, we find that the transport properties are actually affected by Cr impurity scattering, which may induce a metal-to-insulator crossover in highly doped BaFe1.7−yNi0.3CryAs2.
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    Structural and Magnetic Phase Transitions near Optimal Superconductivity in BaFe2(As1−xPx)2
    (American Physical Society, 2015) Hu, Ding; Lu, Xingye; Zhang, Wenliang; Luo, Huiqian; Li, Shiliang; Wang, Peipei; Chen, Genfu; Han, Fei; Banjara, Shree R.; Sapkota, A.; Kreyssig, A.; Goldman, A.I.; Yamani, Z.; Niedermayer, Christof; Skoulatos, Markos; Georgii, Robert; Keller, T.; Wang, Pengshuai; Yu, Weiqiang; Dai, Pengcheng
    We use nuclear magnetic resonance (NMR), high-resolution x-ray, and neutron scattering studies to study structural and magnetic phase transitions in phosphorus-doped BaFe2(As1−xPx)2. Previous transport, NMR, specific heat, and magnetic penetration depth measurements have provided compelling evidence for the presence of a quantum critical point (QCP) near optimal superconductivity at x=0.3. However, we show that the tetragonal-to-orthorhombic structural (Ts) and paramagnetic to antiferromagnetic (AF, TN) transitions in BaFe2(As1−xPx)2 are always coupled and approach TN≈Ts≥Tc (≈29  K) for x=0.29 before vanishing abruptly for x≥0.3. These results suggest that AF order in BaFe2(As1−xPx)2 disappears in a weakly first-order fashion near optimal superconductivity, much like the electron-doped iron pnictides with an avoided QCP.