Browsing by Author "Marquez Peraca, Nicolas"

Now showing 1 - 6 of 6
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    Magnonic superradiant phase transition
    (Springer Nature, 2022) Bamba, Motoaki; Li, Xinwei; Marquez Peraca, Nicolas; Kono, Junichiro
    In the superradiant phase transition (SRPT), coherent light and matter fields are expected to appear spontaneously in a coupled light–matter system in thermal equilibrium. However, such an equilibrium SRPT is forbidden in the case of charge-based light–matter coupling, known as no-go theorems. Here, we show that the low-temperature phase transition of ErFeO3 at a critical temperature of approximately 4 K is an equilibrium SRPT achieved through coupling between Fe3+ magnons and Er3+ spins. By verifying the efficacy of our spin model using realistic parameters evaluated via terahertz magnetospectroscopy and magnetization experiments, we demonstrate that the cooperative, ultrastrong magnon–spin coupling causes the phase transition. In contrast to prior studies on laser-driven non-equilibrium SRPTs in atomic systems, the magnonic SRPT in ErFeO3 occurs in thermal equilibrium in accordance with the originally envisioned SRPT, thereby yielding a unique ground state of a hybrid system in the ultrastrong coupling regime.
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    New Frontiers in Quantum Simulation of an Extended Dicke Model and Active Cooling
    (2023-08-08) Marquez Peraca, Nicolas; Kono, Junichiro
    Groundbreaking discoveries in the fields of light-matter interactions and thermoelectrics in the past two decades have profoundly shaped our understanding of how photons, electrons, and phonons interact. Increased control over the quality of engineered systems, novel measurement techniques, and quantitative improvements in theory are the driving force behind modern, record-high values of light-matter coupling strength and thermoelectric performance. In this work, I bring together experimental and theoretical techniques to study the interplay between magnons and spins in ErFeO3, photons and plasmons in Fischer nanostructures, and electrons and phonons in thermoelectric active cooling materials. Specifically, I perform terahertz time-domain magneto-spectroscopy measurements on the rare-earth orthoferrite ErFeO3 as a function of temperature and magnetic field, and we propose a novel protocol that uses this material as a solid-state quantum simulator of an extended Dicke model. Then, I conduct aperture-based scanning near-field optical microscopy measurements on Fischer nanostructures, and observe field enhancement and localization with resolution beyond the diffraction limit. Lastly, I study active cooling under arbitrary external thermal resistances, and map out the regions where active cooling is advantageous compared to Carnot-limit refrigeration. These results lead to a deeper understanding of fundamental interactions in magnetic, semiconducting, and low-dimensional materials, and further motivate translating research into engineering solutions.
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    Perfect intrinsic squeezing at the superradiant phase transition critical point
    (Springer Nature, 2023) Hayashida, Kenji; Makihara, Takuma; Marquez Peraca, Nicolas; Fallas Padilla, Diego; Pu, Han; Kono, Junichiro; Bamba, Motoaki
    Some of the most exotic properties of the quantum vacuum are predicted in ultrastrongly coupled photon–atom systems; one such property is quantum squeezing leading to suppressed quantum fluctuations of photons and atoms. This squeezing is unique because (1) it is realized in the ground state of the system and does not require external driving, and (2) the squeezing can be perfect in the sense that quantum fluctuations of certain observables are completely suppressed. Specifically, we investigate the ground state of the Dicke model, which describes atoms collectively coupled to a single photonic mode, and we found that the photon–atom fluctuation vanishes at the onset of the superradiant phase transition in the thermodynamic limit of an infinite number of atoms. Moreover, when a finite number of atoms is considered, the variance of the fluctuation around the critical point asymptotically converges to zero, as the number of atoms is increased. In contrast to the squeezed states of flying photons obtained using standard generation protocols with external driving, the squeezing obtained in the ground state of the ultrastrongly coupled photon–atom systems is resilient against unpredictable noise.
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    Quantum simulation of an extended Dicke model with a magnetic solid
    (Springer Nature, 2024) Marquez Peraca, Nicolas; Li, Xinwei; Moya, Jaime M.; Hayashida, Kenji; Kim, Dasom; Ma, Xiaoxuan; Neubauer, Kelly J.; Fallas Padilla, Diego; Huang, Chien-Lung; Dai, Pengcheng; Nevidomskyy, Andriy H.; Pu, Han; Morosan, Emilia; Cao, Shixun; Bamba, Motoaki; Kono, Junichiro
    The Dicke model describes the cooperative interaction of an ensemble of two-level atoms with a single-mode photonic field and exhibits a quantum phase transition as a function of light–matter coupling strength. Extending this model by incorporating short-range atom–atom interactions makes the problem intractable but is expected to produce new physical phenomena and phases. Here, we simulate such an extended Dicke model using a crystal of ErFeO3, where the role of atoms (photons) is played by Er3+ spins (Fe3+ magnons). Through terahertz spectroscopy and magnetocaloric effect measurements as a function of temperature and magnetic field, we demonstrated the existence of a novel atomically ordered phase in addition to the superradiant and normal phases that are expected from the standard Dicke model. Further, we elucidated the nature of the phase boundaries in the temperature–magnetic-field phase diagram, identifying both first-order and second-order phase transitions. These results lay the foundation for studying multiatomic quantum optics models using well-characterized many-body solid-state systems.
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    Terahertz Faraday and Kerr rotation spectroscopy of Bi1−xSbx films in high magnetic fields up to 30 tesla
    (American Physical Society, 2019) Li, Xinwei; Yoshioka, Katsumasa; Xie, Ming; Noe, G. Timothy; Lee, Woojoo; Marquez Peraca, Nicolas; Gao, Weilu; Hagiwara, Toshio; Handegård, Ørjan S.; Nien, Li-Wei; Nagao, Tadaaki; Kitajima, Masahiro; Nojiri, Hiroyuki; Shih, Chih-Kang; MacDonald, Allan H.; Katayama, Ikufumi; Takeda, Jun; Fiete, Gregory A.; Kono, Junichiro
    We report results of terahertz Faraday and Kerr rotation spectroscopy measurements on thin films of Bi1−xSbx, an alloy system that exhibits a semimetal-to-topological-insulator transition as the Sb composition x increases. By using a single-shot time-domain terahertz spectroscopy setup combined with a table-top pulsed minicoil magnet, we conducted measurements in magnetic fields up to 30 T, observing distinctly different behaviors between semimetallic (x<0.07) and topological insulator (x>0.07) samples. Faraday and Kerr rotation spectra for the semimetallic films showed a pronounced dip that blueshifted with the magnetic field, whereas spectra for the topological insulator films were positive and featureless, increasing in amplitude with increasing magnetic field and eventually saturating at high fields (>20 T). Ellipticity spectra for the semimetallic films showed resonances, whereas the topological insulator films showed no detectable ellipticity. To explain these observations, we developed a theoretical model based on realistic band parameters and the Kubo formula for calculating the optical conductivity of Landau-quantized charge carriers. Our calculations quantitatively reproduced all experimental features, establishing that the Faraday and Kerr signals in the semimetallic films predominantly arise from bulk hole cyclotron resonances while the signals in the topological insulator films represent combined effects of surface carriers originating from multiple electron and hole pockets. These results demonstrate that the use of high magnetic fields in terahertz magnetopolarimetry, combined with detailed electronic structure and conductivity calculations, allows us to unambiguously identify and quantitatively determine unique contributions from different species of carriers of topological and nontopological nature in Bi1−xSbx.
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    Ultrastrong magnon–magnon coupling dominated by antiresonant interactions
    (Springer Nature, 2021) Makihara, Takuma; Hayashida, Kenji; Noe Ii, G. Timothy; Li, Xinwei; Marquez Peraca, Nicolas; Ma, Xiaoxuan; Jin, Zuanming; Ren, Wei; Ma, Guohong; Katayama, Ikufumi; Takeda, Jun; Nojiri, Hiroyuki; Turchinovich, Dmitry; Cao, Shixun; Bamba, Motoaki; Kono, Junichiro
    Exotic quantum vacuum phenomena are predicted in cavity quantum electrodynamics systems with ultrastrong light-matter interactions. Their ground states are predicted to be vacuum squeezed states with suppressed quantum fluctuations owing to antiresonant terms in the Hamiltonian. However, such predictions have not been realized because antiresonant interactions are typically negligible compared to resonant interactions in light-matter systems. Here we report an unusual, ultrastrongly coupled matter-matter system of magnons that is analytically described by a unique Hamiltonian in which the relative importance of resonant and antiresonant interactions can be easily tuned and the latter can be made vastly dominant. We found a regime where vacuum Bloch-Siegert shifts, the hallmark of antiresonant interactions, greatly exceed analogous frequency shifts from resonant interactions. Further, we theoretically explored the system’s ground state and calculated up to 5.9 dB of quantum fluctuation suppression. These observations demonstrate that magnonic systems provide an ideal platform for exploring exotic quantum vacuum phenomena predicted in ultrastrongly coupled light-matter systems.