Browsing by Author "Jin, Changqing"

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    Disentangling superconducting and magnetic orders in NaFe1−xNixAs using muon spin rotation
    (American Physical Society, 2018) Cheung, Sky C.; Guguchia, Zurab; Frandsen, Benjamin A.; Gong, Zizhou; Yamakawa, Kohtaro; Almeida, Dalson E.; Onuorah, Ifeanyi J.; Bonfá, Pietro; Miranda, Eduardo; Wang, Weiyi; Tam, David W.; Song, Yu; Cao, Chongde; Cai, Yipeng; Hallas, Alannah M.; Wilson, Murray N.; Munsie, Timothy J.S.; Luke, Graeme; Chen, Bijuan; Dai, Guangyang; Jin, Changqing; Guo, Shengli; Ning, Fanlong; Fernandes, Rafael M.; De Renzi, Roberto; Dai, Pengcheng; Uemura, Yasutomo J.
    Muon spin rotation and relaxation studies have been performed on a “111” family of iron-based superconductors, NaFe1−xNixAs, using single crystalline samples with Ni concentrations x=0, 0.4, 0.6, 1.0, 1.3, and 1.5%. Static magnetic order was characterized by obtaining the temperature and doping dependences of the local ordered magnetic moment size and the volume fraction of the magnetically ordered regions. For x=0 and 0.4%, a transition to a nearly-homogeneous long range magnetically ordered state is observed, while for x≳0.4% magnetic order becomes more disordered and is completely suppressed for x=1.5%. The magnetic volume fraction continuously decreases with increasing x. Development of superconductivity in the full volume is inferred from Meissner shielding results for x≳0.4%. The combination of magnetic and superconducting volumes implies that a spatially-overlapping coexistence of magnetism and superconductivity spans a large region of the T−x phase diagram for NaFe1−xNixAs. A strong reduction of both the ordered moment size and the volume fraction is observed below the superconducting TC for x=0.6, 1.0, and 1.3%, in contrast to other iron pnictides in which one of these two parameters exhibits a reduction below TC, but not both. The suppression of magnetic order is further enhanced with increased Ni doping, leading to a reentrant nonmagnetic state below TC for x=1.3%. The reentrant behavior indicates an interplay between antiferromagnetism and superconductivity involving competition for the same electrons. These observations are consistent with the sign-changing s± superconducting state, which is expected to appear on the verge of microscopic coexistence and phase separation with magnetism. We also present a universal linear relationship between the local ordered moment size and the antiferromagnetic ordering temperature TN across a variety of iron-based superconductors. We argue that this linear relationship is consistent with an itinerant-electron approach, in which Fermi surface nesting drives antiferromagnetic ordering. In studies of superconducting properties, we find that the T=0 limit of superfluid density follows the linear trend observed in underdoped cuprates when plotted against TC. This paper also includes a detailed theoretical prediction of the muon stopping sites and provides comparisons with experimental results.
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    Magnetic moment evolution and spin freezing in doped BaFe2As2
    (Springer Nature, 2017) Pelliciari, Jonathan; Huang, Yaobo; Ishii, Kenji; Zhang, Chenglin; Dai, Pengcheng; Chen, Gen Fu; Xing, Lingyi; Wang, Xiancheng; Jin, Changqing; Ding, Hong; Werner, Philipp; Schmitt, Thorsten
    Fe-K β X-ray emission spectroscopy measurements reveal an asymmetric doping dependence of the magnetic moments μbare in electron- and hole-doped BaFe2As2. At low temperature, μbare is nearly constant in hole-doped samples, whereas it decreases upon electron doping. Increasing temperature substantially enhances μbare in the hole-doped region, which is naturally explained by the theoretically predicted crossover into a spin-frozen state. Our measurements demonstrate the importance of Hund’s-coupling and electronic correlations, especially for hole-doped BaFe2As2, and the inadequacy of a fully localized or fully itinerant description of the 122 family of Fe pnictides.
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    Orbital Selective Spin Excitations and their Impact on Superconductivity of LiFe1−xCoxAs
    (American Physical Society, 2016) Li, Yu; Yin, Zhiping; Wang, Xiancheng; Tam, David W.; Abernathy, D.L.; Podlesnyak, A.; Zhang, Chenglin; Wang, Meng; Xing, Lingyi; Jin, Changqing; Haule, Kristjan; Kotliar, Gabriel; Maier, Thomas A.; Dai, Pengcheng
    We use neutron scattering to study spin excitations in single crystals of LiFe0.88Co0.12As, which is located near the boundary of the superconducting phase of LiFe1−xCoxAs and exhibits non-Fermi-liquid behavior indicative of a quantum critical point. By comparing spin excitations of LiFe0.88Co0.12As with a combined density functional theory and dynamical mean field theory calculation, we conclude that wave-vector correlated low energy spin excitations are mostly from the dxy orbitals, while high-energy spin excitations arise from the dyz and dxz orbitals. Unlike most iron pnictides, the strong orbital selective spin excitations in the LiFeAs family cannot be described by an anisotropic Heisenberg Hamiltonian. While the evolution of low-energy spin excitations of LiFe1−xCoxAs is consistent with the electron-hole Fermi surface nesting conditions for the dxy orbital, the reduced superconductivity in LiFe0.88Co0.12As suggests that Fermi surface nesting conditions for the dyz and dxz orbitals are also important for superconductivity in iron pnictides.