Browsing by Author "Ishii, Kenji"

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    Magnetic moment evolution and spin freezing in doped BaFe2As2
    (Springer Nature, 2017) Pelliciari, Jonathan; Huang, Yaobo; Ishii, Kenji; Zhang, Chenglin; Dai, Pengcheng; Chen, Gen Fu; Xing, Lingyi; Wang, Xiancheng; Jin, Changqing; Ding, Hong; Werner, Philipp; Schmitt, Thorsten
    Fe-K β X-ray emission spectroscopy measurements reveal an asymmetric doping dependence of the magnetic moments μbare in electron- and hole-doped BaFe2As2. At low temperature, μbare is nearly constant in hole-doped samples, whereas it decreases upon electron doping. Increasing temperature substantially enhances μbare in the hole-doped region, which is naturally explained by the theoretically predicted crossover into a spin-frozen state. Our measurements demonstrate the importance of Hund’s-coupling and electronic correlations, especially for hole-doped BaFe2As2, and the inadequacy of a fully localized or fully itinerant description of the 122 family of Fe pnictides.