Browsing by Author "Frandsen, B."

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    An itinerant antiferromagnetic metal without magnetic constituents
    (Nature Publishing Group, 2015) Svanidze, E.; Wang, Jiakui K.; Besara, T.; Liu, L.; Huang, Q.; Siegrist, T.; Frandsen, B.; Lynn, J.W.; Nevidomskyy, Andriy H.; Gamża, Monika B.; Aronson, M.C.; Uemura, Y.J.; Morosan, E.
    The origin of magnetism in metals has been traditionally discussed in two diametrically opposite limits: itinerant and local moments. Surprisingly, there are very few known examples of materials that are close to the itinerant limit, and their properties are not universally understood. In the case of the two such examples discovered several decades ago, the itinerant ferromagnets ZrZn2 and Sc3In, the understanding of their magnetic ground states draws on the existence of 3d electrons subject to strong spin fluctuations. Similarly, in Cr, an elemental itinerant antiferromagnet with a spin density wave ground state, its 3d electron character has been deemed crucial to it being magnetic. Here, we report evidence for an itinerant antiferromagnetic metal with no magnetic constituents: TiAu. Antiferromagnetic order occurs below a Néel temperature of 36 K, about an order of magnitude smaller than in Cr, rendering the spin fluctuations in TiAu more important at low temperatures. This itinerant antiferromagnet challenges the currently limited understanding of weak itinerant antiferromagnetism, while providing insights into the effects of spin fluctuations in itinerant–electron systems.
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    Non-Fermi Liquid Behavior Close to a Quantum Critical Point in a Ferromagnetic State without Local Moments
    (American Physical Society, 2015) Svanidze, E.; Liu, L.; Frandsen, B.; White, B.D.; Besara, T.; Goko, T.; Medina, T.; Munsie, T.J.S.; Luke, G.M.; Zheng, D.; Jin, C.Q.; Siegrist, T.; Maple, M.B.; Uemura, Y.J.; Morosan, E.
    A quantum critical point (QCP) occurs upon chemical doping of the weak itinerant ferromagnet Sc3.1In. Remarkable for a system with no local moments, the QCP is accompanied by non-Fermi liquid behavior, manifested in the logarithmic divergence of the specific heat both in the ferro-and the paramagnetic states, as well as linear temperature dependence of the low-temperature resistivity. With doping, critical scaling is observed close to the QCP, as the critical exponents δ, γ, and β have weak composition dependence, with δ nearly twice and β almost half of their respective mean-field values. The unusually large paramagnetic moment μPM∼1.3μB/F.U. is nearly composition independent. Evidence for strong spin fluctuations, accompanying the QCP at xc=0.035±0.005, may be ascribed to the reduced dimensionality of Sc3.1In, associated with the nearly one-dimensional Sc-In chains.