Rice University Research Repository
The Rice Research Repository (R-3) provides access to research produced at Rice University, including theses and dissertations, journal articles, research center publications, datasets, and academic journals. Managed by Fondren Library, R-3 is indexed by Google and Google Scholar, follows best practices for preservation, and provides DOIs to facilitate citation. Woodson Research Center collections, including Rice Images and Documents and the Task Force on Slavery, Segregation, and Racial Injustice, have moved here.
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Multicomponent plasmonic photocatalysts consisting of a plasmonic antenna and a reactive catalytic surface: the antenna-reactor effect
(2024-10-08) Halas, Nancy Jean; Nordlander, Peter; Robatjazi, Hossein; Swearer, Dayne Francis; Zhang, Chao; Zhao, Hangqi; Zhou, Linan; Rice University; United States Patent and Trademark Office
A multicomponent photocatalyst includes a reactive component optically, electronically, or thermally coupled to a plasmonic material. A method of performing a catalytic reaction includes loading a multicomponent photocatalyst including a reactive component optically, electronically, or thermally coupled to a plasmonic material into a reaction chamber; introducing molecular reactants into the reaction chamber; and illuminating the reaction chamber with a light source.
The Okjökull Memorial and Geohuman Relations
(Berghahn Books, 2024) Howe, Cymene; Boyer, Dominic
Focusing on the life and death of Okjökull, the first of Iceland's major glaciers to disappear because of anthropogenic climate change, this article discusses the complex relationships between cryospheres and human communities in Iceland. It asks how distinctions between non-living entities and living beings can offer insights to anthropology, and transdisciplinarily, as a model for recognising mutual precarities between the living and non-living world in the face of anthropogenic climate change. Detailing the authors’ ethnographic encounters with Ok mountain and Okjökull (glacier), the authors argue that by attending to non-living forms, and by registering their ‘passing’ or loss, we are able to document and better comprehend threshold events in the larger life of the planet. Résumé En se concentrant sur la vie et la mort d'Okjökull, le premier des principaux glaciers islandais à disparaître en raison des changements climatiques anthropogéniques, cet article discute les relations complexes entre la cryosphère et les communautés humaines en Islande. Il questionne la manière dont les distinctions entre entités non vivantes et êtres vivants peuvent offrir des perspectives à l'anthropologie et la transdisciplinarité en tant que modèle pour reconnaitre des précarités mutuelles entre monde vivant et non vivant en face du changement climatique anthropogénique. En détaillant la rencontre ethnographique entre les auteurs, la montagne Ok et l'Okjökull (le glacier), les auteurs défendent l'idée qu'en prenant acte des formes non vivantes et en marquant leur « disparition » ou leur perte, nous sommes en mesure de documenter et de mieux comprendre les événements de bascule dans la vie de notre planète.
Single-cell somatic copy number variants in brain using different amplification methods and reference genomes
(Springer Nature, 2024) Kalef-Ezra, Ester; Turan, Zeliha Gozde; Perez-Rodriguez, Diego; Bomann, Ida; Behera, Sairam; Morley, Caoimhe; Scholz, Sonja W.; Jaunmuktane, Zane; Demeulemeester, Jonas; Sedlazeck, Fritz J.; Proukakis, Christos
The presence of somatic mutations, including copy number variants (CNVs), in the brain is well recognized. Comprehensive study requires single-cell whole genome amplification, with several methods available, prior to sequencing. Here we compare PicoPLEX with two recent adaptations of multiple displacement amplification (MDA): primary template-directed amplification (PTA) and droplet MDA, across 93 human brain cortical nuclei. We demonstrate different properties for each, with PTA providing the broadest amplification, PicoPLEX the most even, and distinct chimeric profiles. Furthermore, we perform CNV calling on two brains with multiple system atrophy and one control brain using different reference genomes. We find that 20.6% of brain cells have at least one Mb-scale CNV, with some supported by bulk sequencing or single-cells from other brain regions. Our study highlights the importance of selecting whole genome amplification method and reference genome for CNV calling, while supporting the existence of somatic CNVs in healthy and diseased human brain.
Three-dimensional printing of wood
(AAAS, 2024) Thakur, Md Shajedul Hoque; Shi, Chen; Kearney, Logan T.; Saadi, M. A. S. R.; Meyer, Matthew D.; Naskar, Amit K.; Ajayan, Pulickel M.; Rahman, Muhammad M.
Natural wood has served as a foundational material for buildings, furniture, and architectural structures for millennia, typically shaped through subtractive manufacturing techniques. However, this process often generates substantial wood waste, leading to material inefficiency and increased production costs. A potential opportunity arises if complex wood structures can be created through additive processes. Here, we demonstrate an additive-free, water-based ink made of lignin and cellulose, the primary building blocks of natural wood, that can be used to three-dimensional (3D) print architecturally designed wood structures via direct ink writing. The resulting printed structures, after heat treatment, closely resemble the visual, textural, olfactory, and macro-anisotropic properties, including mechanical properties, of natural wood. Our results pave the way for 3D-printed wooden construction with a sustainable pathway to upcycle/recycle natural wood.
Spontaneous reversal of spin chirality and competing phases in the topological magnet EuAl4
(Springer Nature, 2024) Vibhakar, Anuradha M.; Khalyavin, Dmitry D.; Orlandi, Fabio; Moya, Jamie M.; Lei, Shiming; Morosan, Emilia; Bombardi, Alessandro
Materials exhibiting a spontaneous reversal of spin chirality have the potential to drive the widespread adoption of chiral magnets in spintronic devices. Unlike the majority of chiral magnets that require the application of an external field to reverse the spin chirality, we observe the spin chirality to spontaneously reverse in the topological magnet EuAl4. Using resonant elastic x-ray scattering we demonstrate that all four magnetic phases in EuAl4 are single-k, where the first two magnetic phases are characterized by spin density wave order and the last two by helical spin order. A single spin chirality was stabilised across the 1mm2 sample, and the reversal of spin chirality occurred whilst maintaining a helical magnetic structure. At the onset of the helical magnetism, the crystal symmetry lowers to a chiral monoclinic space group, explaining the asymmetry in the chiral spin order, and establishing a mechanism by which the spin chirality could reverse via magnetostructural coupling.